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Author(s) |
Yusuf, S. M.; Bera, A. K.; Kini, N. S.; Mirebeau, I.; Petit, S. |
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The magnetic correlations in the quasi-two-dimensional (2D) spin-
½
square-lattice system Zn2VO(PO4)2 have been investigated by neutron-diffraction technique. A long-range antiferromagnetic (AFM) ordering below 3.75 K (TN) has been observed with a reduced moment of 0.66 (2)
µB per V ion at 1.5 K. In a given ab plane, the AFM spin arrangement is Néel type and the AFM layers are coupled ferromagnetically along the c axis. Remarkably, we have observed a pure 2D short-range AFM ordering in the
ab plane above TN. Interestingly, the coexistence of diffuse magnetic scattering and three-dimensional antiferromagnetic Bragg peaks has been found below TN, indicating the presence of spin waves as confirmed by our calculation using the linear spin-wave theory. The observed results are discussed in the light of existing theory for a two-dimensional spin-
½ square-lattice system. |
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