BARC/PUB/10//0819

 
 

Two-and three-dimensional magnetic correlations in the spin- 1/2 square-lattice system Zn2VO(PO4)2

 
     
 
Author(s)

Yusuf, S. M.; Bera, A. K.; Kini, N. S.; Mirebeau, I.; Petit, S.

ABSTRACT

The magnetic correlations in the quasi-two-dimensional (2D) spin- ½ square-lattice system Zn2VO(PO4)2 have been investigated by neutron-diffraction technique. A long-range antiferromagnetic (AFM) ordering below 3.75 K (TN) has been observed with a reduced moment of 0.66 (2) µB per V ion at 1.5 K. In a given ab plane, the AFM spin arrangement is Néel type and the AFM layers are coupled ferromagnetically along the c axis. Remarkably, we have observed a pure 2D short-range AFM ordering in the ab plane above TN. Interestingly, the coexistence of diffuse magnetic scattering and three-dimensional antiferromagnetic Bragg peaks has been found below TN, indicating the presence of spin waves as confirmed by our calculation using the linear spin-wave theory. The observed results are discussed in the light of existing theory for a two-dimensional spin-  ½ square-lattice system.

 
 
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