BARC/PUB/2015/0595

 
 

Understanding photoexcitation dynamics in a three-step photoionization of atomic uranium and measurement of photoexcitation and photoionization cross sections

 
     
 
Author(s)

Mandal, P. K.; Sahoo, A. C.; Das, R. C.; Shah, M. L.; Pulhani, A. K.; Manohar, K. G.; Dev, V.
(L&PTD)

Source

Applied Physics-B, 2015. Vol. 120 (4): pp. 751-758

ABSTRACT

Photo excitation dynamics in a three-step photo ionization of atomic uranium has been investigated using time-resolved two-color three-photon and delayed three-color three-photon photo ionization signals. Investigations are carried out in an atomic beam of uranium coupled to a high-resolution time-of-flight mass spectrometer using three tunable pulsed dye lasers. Dependence of both the signals on the second-step laser photon fluence is studied. Excited-level-to-excited-level photo excitation cross section and photo ionization cross section from the second excited level are simultaneously determined by analyzing the two-color three-photon and three-color three-photon photo ionization signals using population rate equation model. Using this methodology, photo excitation and photo ionization cross sections at seven values of the second-step laser wavelength have been measured. From the measured values of the photo excitation cross sections, we have obtained excited-level-to-excited-level transition probabilities and compared these with the values reported in the literature.

 
 
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