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Author(s) |
Yogesh Kumar; Bhatt, H.; Prajapat, C. L.; Poswal, H. K.; Basu, S.; Singh, S. (SSPD;TSD;HP&SRPD)
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Source |
Journal of Applied Physics, 2018. Vol. 124: Article no. 065302 |
ABSTRACT
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We have deposited LaNiO3 thin films on LaAlO3 (001), SrTiO3 (001), and Si (001) substrates using the pulsed laser deposition technique. Depositions were carried out at various substrate temperatures ranging from 0 to 800 oC. The effects of lattice mismatch and structural disorder on the transport properties of films deposited on various substrates and at different substrate temperatures are reported. X-ray diffraction confirms a highly c-axis oriented growth of LaNiO3 films on all the substrates at substrate temperatures of 600 and 800 oC, while at lower substrate temperatures deposited films are amorphous. Emergence of a new Raman mode indicates symmetry lowering in all the deposited crystalline films. Hardening of the Eg(3) (~400 cm-1) mode is also observed with the rise of in-plane compressive strain. Resistivity curves for films on Si show a semiconducting behaviour and follow a variable range hopping mechanism. Crystalline films on LaAlO3 and SrTiO3 exhibit a metallic character along with a low-temperature resistivity upturn, which is attributed to the contribution of self-localization to resistivity at low temperatures as indicated by magnetotransport measurements. |
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